The ATMONSYS water vapor DIAL: advanced measurements of short-term variability in the planetary boundary layer

Abstract

High-resolution measurements of water vapor concentrations and their transport throughout the turbulent planetary boundary layer (PBL) and beyond are key for an enhanced understanding of atmospheric processes. This study presents data from the mobile Atmospheric Monitoring System (ATMONSYS) Differential Absorption Lidar (DIAL), operated with a novel titanium sapphire (Ti:Sa) laser concept, for the first time. The ATMONSYS DIAL aims to resolve turbulence throughout the PBL with a sampling frequency of 10 sand vertical resolutions of less than 200 m. General measuring capabilities during high-noon, clear-sky, summer conditions with a maximum vertical measurement range of >3 km and statistical uncertainties of <5 % are demonstrated. The analysis of turbulence spectra shows good agreement with Kolmogorov's law, demonstrating the system's capability to resolve turbulence. However, deviations from Kolmogorov behavior are observed at certain frequency ranges. By combining the ATMONSYS DIAL with an adjacent high-quality Doppler wind lidar, some of these deviations are mitigated in the co-spectra due to independent noise from both instruments. However, intermediate deviations from Kolmogorov behavior persist, likely due to surrounding surface heterogeneities. The agreement of the co-spectra with Kolmogorov's law at the highest frequencies demonstrates that the ATMONSYS DIAL is capable of resolving turbulent latent energy fluxes down to the measurement's Nyquist frequency of 5×10-2Hz. A system cross-intercomparison of the ATMONSYS DIAL with two adjacent water vapor Raman lidars and radiosondes shows overall good agreement between the sensors, despite minor DIAL deficiencies under certain conditions with broken clouds passing over the lidar. The observed profile-to-profile DIAL fluctuations and sensor-to-sensor deviations, in combination with low statistical uncertainty, highlight the advantage of humidity lidars, such as the ATMONSYS DIAL, in capturing both short-term and small-scale dynamics of the lowermost atmosphere.